Controlling the shape morphology of origami-inspired photoresponsive hydrogels.
Controlling the shape morphology of origami-inspired photoresponsive hydrogels.
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DOI:
10.1039/d1sm01751a
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发表时间:
2022-03-16
期刊:
影响因子:
3.4
通讯作者:
Olvera de la Cruz M
中科院分区:
文献类型:
--
作者:
Aggarwal A;Li C;Stupp SI;Olvera de la Cruz M
The concept of origami has influenced the development of responsive materials that can mimic complex functions performed by living organisms. An ultimate goal is to discover and design soft materials that can be remotely actuated into diverse structures. To achieve this goal, we design and synthesize here a light-responsive spiropyran hydrogel system that can display dynamic shape changes upon irradiation with local light. We use a continuum polymer model to analyze the behavior of the constructed photoactive hydrogel, which is in good agreement with the experimental results. We explore different buckling modalities and patterns in a different range of parameters. The synthesis and fabrication of these materials demonstrate that the theoretical model can be used to drive the development of responsive photoactive systems.
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