Catalytic methane oxidation at low temperatures using ozone

Catalytic methane oxidation at low temperatures using ozone
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使用臭氧在低温下催化甲烷氧化

DOI:
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发表时间:
1996
期刊:
影响因子:
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通讯作者:
S. Oyama
S. Oyama
中科院分区:
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文献类型:
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作者:
W. Li;S. Oyama

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本文详细研究了在较低温度(<450°C)下,以臭氧或氧气为氧化剂的甲烷氧化反应。已给予适当的注意,以建立气相反应的作用。监测反应前后的臭氧和甲烷浓度,以确定反应的化学计量和可能涉及的链式反应。MgO被用作该反应的催化剂。
This paper reports a detailed study of methane oxidation at relatively low temperatures (<450°C) using ozone or oxygen as the oxidizing agents. Due attention has been given to establish the role of gas phase reactions. The ozone and methane concentrations before and after the reaction were monitored to determine the stoichiometry of the reaction and the possible involvement of chain reactions. MgO was used as a catalyst for this reaction.