Ultrafast collective dynamics in the charge-density-wave conductor K(0.3)MoO(3).

Ultrafast collective dynamics in the charge-density-wave conductor K(0.3)MoO(3).
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电荷密度波导体 K(0.3)MoO(3) 中的超快集体动力学。

DOI:
10.1063/1.1645785
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发表时间:
2003
期刊:
The Journal of chemical physics
影响因子:
--
通讯作者:
G. Lupke
G. Lupke
中科院分区:
--
文献类型:
--
作者:
Yuhang Ren;Zhu;G. Lupke

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用飞秒泵浦探测光谱研究了蓝青铜(K(0.3)MoO(3))和红青铜(K(0.33)MoO(3))中低能相干电荷密度波的激发。在K(0.33)MoO(3)中观察到具有明显各向异性的横向相的线性无间隙、类声色散关系。在30k时,振幅模式表现出微弱的色散关系,频率为1.67太赫兹。我们的结果首次表明,时间分辨光学技术提供了强相关电子系统中集体激发的动量分辨。
Low-energy coherent charge-density wave excitations are investigated in blue bronze (K(0.3)MoO(3)) and red bronze (K(0.33)MoO(3)) by femtosecond pump-probe spectroscopy. A linear gapless, acousticlike dispersion relation is observed for the transverse phasons with a pronounced anisotropy in K(0.33)MoO(3). The amplitude mode exhibits a weak (opticlike) dispersion relation with a frequency of 1.67 THz at 30 K. Our results show for the first time that the time-resolved optical technique provides momentum resolution of collective excitations in strongly correlated electron systems.