On Process Intensification through Membrane Storage Reactors
On Process Intensification through Membrane Storage Reactors
复制标题
通过膜储存反应器进行过程强化
作者：
J. Iii;T. Tsotsis;V. Manousiouthakis
在这项工作中，开发并模拟了新型膜存储反应器（MSR）过程的动态、一维、基于第一原理的模型。由此产生的控制方程被呈现为无量纲，并显示出具有两个可用于影响过程性能的无量纲组的特征。该新颖的过程被证明可以通过创建由半渗透边界分隔的两个物理上不同的域和动态操作来强化所需物种的生产。然后介绍了许多指标并将其应用于蒸汽甲烷重整的案例研究，为此进行了参数研究，确定了 MSR 与稳态 (SSR) 运行的反应器相比具有优越的性能。
In this work, a dynamic, one-dimensional, first principle-based model of a novel membrane storage reactor (MSR) process is developed and simulated. The resulting governing equations are rendered dimensionless and are shown to feature two dimensionless groups that can be used to affect process performance. The novel process is shown to intensify production of a desired species through the creation of two physically distinct domains separated by a semipermeable boundary, and dynamic operation. A number of metrics are then introduced and applied to a case study on Steam Methane Reforming, for which a parametric study is carried out which establishes the superior performance of the MSR when compared to a reactor operating at steady state (SSR).