Nearly logarithmic decay of correlations in glass-forming liquids -: art. no. 105701

Nearly logarithmic decay of correlations in glass-forming liquids -: art. no. 105701
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DOI:
10.1103/physrevlett.92.105701
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发表时间:
2004-03-12
影响因子:
8.6
通讯作者:
Sperl, M
Sperl, M
中科院分区:
物理与天体物理1区
文献类型:
--
作者:
Götze, W;Sperl, M

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Nearly logarithmic decay of correlations, which was observed for several supercooled liquids in optical-Kerr-effect experiments [G. Hinze et al., Phys. Rev. Lett. 84, 2437 (2000); H. Cang et al., Phys. Rev. Lett. 90, 197401 (2003)], is explained within the mode-coupling theory for ideal glass transitions as a manifestation of the beta-peak phenomenon. A schematic model, which describes the dynamics by only two correlators, one referring to density fluctuations and the other to the reorientational fluctuations of the molecules, yields for strong rotation-translation coupling response functions in agreement with those measured for benzophenone and Salol for the time interval extending from 2 ps to about 20 and 200 ns, respectively.