Connecting glass-forming ability of binary mixtures of soft particles to equilibrium melting temperatures
Connecting glass-forming ability of binary mixtures of soft particles to equilibrium melting temperatures
复制标题
将软颗粒二元混合物的玻璃形成能力与平衡熔化温度联系起来
DOI：
10.1038/s41467-020-16986-z
复制
发表时间：
2020-06
影响因子：
16.6
通讯作者：
Xu Ning
中科院分区：
文献类型：
--
作者：
Nie Yunhuan;Liu Jun;Guo Jialing;Xu Ning
玻璃形成能力是制造玻璃以及理解长期存在的玻璃转变问题的一项重要材料特性。由于其非平衡性质，很难为其建立理论。在此我们报道……
The glass-forming ability is an important material property for manufacturing glasses and understanding the long-standing glass transition problem. Because of the nonequilibrium nature, it is difficult to develop the theory for it. Here we report that the glass-forming ability of binary mixtures of soft particles is related to the equilibrium melting temperatures. Due to the distinction in particle size or stiffness, the two components in a mixture effectively feel different melting temperatures, leading to a melting temperature gap. By varying the particle size, stiffness, and composition over a wide range of pressures, we establish a comprehensive picture for the glass-forming ability, based on our finding of the direct link between the glass-forming ability and the melting temperature gap. Our study reveals and explains the pressure and interaction dependence of the glass-forming ability of model glass-formers, and suggests strategies to optimize the glass-forming ability via the manipulation of particle interactions.
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DOI：
10.1103/physreve.82.060501
发表时间：
2010-09
期刊：
Physical review. E, Statistical, nonlinear, and soft matter physics
影响因子：
--
作者：
L. Berthier;A. Moreno;G. Szamel
通讯作者：
L. Berthier;A. Moreno;G. Szamel
影响因子：
8.6
作者：
Cang Zhao;Kaiwen Tian;N. Xu
通讯作者：
Cang Zhao;Kaiwen Tian;N. Xu
影响因子：
64.8
作者：
Li, Pilong;Banjade, Sudeep;Cheng, Hui-Chun;Kim, Soyeon;Chen, Baoyu;Guo, Liang;Llaguno, Marc;Hollingsworth, Javoris V.;King, David S.;Banani, Salman F.;Russo, Paul S.;Jiang, Qiu-Xing;Nixon, B. Tracy;Rosen, Michael K.
通讯作者：
Rosen, Michael K.
DOI：
10.1103/physreve.87.052310
发表时间：
2013-05
期刊：
Physical review. E, Statistical, nonlinear, and soft matter physics
影响因子：
--
作者：
M. Schmiedeberg
通讯作者：
M. Schmiedeberg
影响因子：
64.8
作者：
S. Sastry;P. Debenedetti;F. Stillinger
通讯作者：
S. Sastry;P. Debenedetti;F. Stillinger