Application of imaging plate technique for separate detection of 3H and 14C

Application of imaging plate technique for separate detection of 3H and 14C
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DOI:
10.1016/j.fusengdes.2005.08.080
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发表时间:
2006-02
影响因子:
1.7
通讯作者:
K. Sugiyama;T. Tanabe;T. Saze;K. Nishizawa
K. Sugiyama;T. Tanabe;T. Saze;K. Nishizawa
中科院分区:
工程技术3区
文献类型:
--
作者:
K. Sugiyama;T. Tanabe;T. Saze;K. Nishizawa

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一种使用14c(一种β衰变放射性同位素)的示踪技术正在计划中,以了解核聚变装置中的碳迁移行为。成像板(IP)是一种成功应用于等离子体壁氚分析的辐射图像探测器,它可以很容易地检测到14c中的β-电子,并给出详细的14c沉积剖面,因此IP方法可以作为14c沉积的死后测量方法之一。然而,由于氚的β-电子会叠加14c的β-电子,因此区分14c的β-电子和氚的β-电子是必要的。为了做到这一点,我们开发了一种薄膜插入技术,在样品和IP之间插入薄膜,以阻止低能量电子通过薄膜。发现可以检测到低至10Bq/cm2(~ 2.6×101214C/cm2)的14c浓度,这表明该技术保持了14c作为高灵敏度示踪剂的优势,并且可以在不受共存氚干扰的情况下进行二维14c谱分析。
A tracer technique using14C, which is a β-decaying radioactive isotope, is being planed to understand the carbon migration behavior in fusion devices. An imaging plate (IP), which is a radiation image detector successfully applied for the tritium analysis of plasma-facing walls, easily detects β-electrons from14C and would give a detailed14C deposition profiles, hence the IP method can be one of the postmortem measurements of the14C deposition. However, since β-electrons from tritium would superpose those from14C, it is essential to differentiate β-electrons of14C from those of tritium. To do this, we have developed a film insertion technique in which a thin film is inserted between a specimen and IP to prohibit lower energy electrons passing through the film. It is found that14C concentrations as small as 10Bq/cm2(∼2.6×101214C/cm2) can be detected, indicating that this technique keeps the advantage of14C as a high sensitivity tracer, and making two-dimensional14C profiling possible without any disturbance of co-existing tritium.