Molecular information processing in nonequilibrium copolymerizations
Molecular information processing in nonequilibrium copolymerizations
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DOI：
10.1063/1.3050099
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发表时间：
2009-01-07
影响因子：
4.4
通讯作者：
Gaspard, Pierre
中科院分区：
文献类型：
--
作者：
Andrieux, David;Gaspard, Pierre
我们认为一般波动共聚过程中，有或没有潜在的模板。我们研究了由非平衡条件引起的空间有序性以及模板和合成共聚物之间的信息传递。信息传输原来是最佳的无限耗散限制时，单体之间没有相关性。相比之下，我们表明，优化制度的信息生成时，模板和相关性的影响相互作用可能存在。
We consider general fluctuating copolymerization processes, with or without underlying templates. We study the spatial ordering resulting from the nonequilibrium conditions as well as the information transmitted between the template and the synthesized copolymer. Information transmission turns out to be optimal in the infinite-dissipation limit when no correlations between the monomers are present. By contrast, we show that optimized regimes of information generation may exist when template and correlations effects interact.