A percolation dynamic approach to the sol-gel transition

A percolation dynamic approach to the sol-gel transition
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溶胶-凝胶转变的渗滤动态方法

DOI:
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发表时间:
1998
期刊:
影响因子:
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通讯作者:
A. Coniglio
A. Coniglio
中科院分区:
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文献类型:
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作者:
E. Gado;L. Arcangelis;A. Coniglio

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在渗流模型中引入键涨落动力学,研究了Sol-Gel转变过程,考察了Sol-Gel的静态和动态性质。在正方形晶格上的计算机模拟表明,其静态性质符合随机渗流模型,自扩散系数在渗流阈值处为零。根据自扩散系数,确定了溶胶-凝胶转变过程中粘度的临界行为,给出了一个指数。
The sol-gel transition is studied introducing the bond fluctuation dynamics within the percolation model in order to investigate both static and dynamic properties. Computer simulations on a square lattice have shown that the static properties agree with the random percolation model and the self-diffusion coefficients vanish at the percolation threshold. From the self-diffusion coefficients the critical behaviour of the viscosity at the sol-gel transition is determined, giving an exponent .