Kinetic Pattern Formation with Intermolecular Interactions: A Modified Brusselator Model

Kinetic Pattern Formation with Intermolecular Interactions: A Modified Brusselator Model
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分子间相互作用的动力学模式形成:改进的 Brusselator 模型

DOI:
10.1007/s10118-021-2600-5
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发表时间:
2021-07-05
影响因子:
4.3
通讯作者:
Yang, Yu-Liang
Yang, Yu-Liang
中科院分区:
化学2区
文献类型:
--
作者:
Sun, Rui-Qi;Li, Jian-Feng;Yang, Yu-Liang

文献摘要

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本文对传统的量子阱模型进行了改进,引入了分子间相互作用,并在此基础上对化学反应和相分离介导的图案形成进行了系统的研究。结果表明,如果相分离占主导地位,则在一定条件下,化学反应将阻止畴尺寸的增长,从而导致耗散结构而不是宏观相分离。
In this work, we modify the traditional Brusselator model to incorporate the intermolecular interactions, based on which a systematic study is performed on the pattern formation mediated by chemical reaction and phase separation. It is found that if the chemical reaction dominates, the pattern formation will be inhibited by the phase separation while if the phase separation dominates, the chemical reaction will prevent, under certain conditions, the domain size from growing which results in dissipative patterns other than macroscopic phase separations.