Maximizing precision in saturation-limited absorption measurements

Maximizing precision in saturation-limited absorption measurements
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DOI:
10.1103/physreva.104.053717
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发表时间:
2021-11-22
期刊:
影响因子:
2.9
通讯作者:
Allen, Euan J.
Allen, Euan J.
中科院分区:
物理与天体物理2区
文献类型:
--
作者:
Biele, Jake;Wollmann, Sabine;Allen, Euan J.

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Quantum fluctuations in the intensity of an optical probe is noise which limits measurement precision in absorption spectroscopy. Increased probe power can offer greater precision; however, this strategy is often constrained by sample saturation. Here, we analyze measurement precision for a generalized absorption model in which we account for saturation and explore its effect on both classical and quantum probe performance. We present a classical probe-sample optimization strategy to maximize precision and find that optimal probe powers always fall within the saturation regime. We apply our optimization strategy to two examples, high-precision Doppler broadened thermometry and an absorption spectroscopy measurement of chlorophyll a. We derive a limit on the maximum precision gained from using a nonclassical probe and find a strategy capable of saturating this bound. We evaluate amplitude-squeezed light as a viable experimental probe state and find it capable of providing precision that reaches to within > 85% of the ultimate quantum limit with currently available technology.