Effects of water addition on the combustion of iso-octane investigated in laminar flames, low-temperature reactors, and an HCCI engine

Effects of water addition on the combustion of iso-octane investigated in laminar flames, low-temperature reactors, and an HCCI engine
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DOI:
10.1016/j.combustflame.2019.11.023
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发表时间:
2020-02
影响因子:
4.4
通讯作者:
Steffen Schmitt;Maximilian Wick;Christian Wouters;L. Ruwe;Isabelle Graf;J. Andert;N. Hansen;S. Pisc
Steffen Schmitt;Maximilian Wick;Christian Wouters;L. Ruwe;Isabelle Graf;J. Andert;N. Hansen;S. Pisc
中科院分区:
工程技术2区
文献类型:
--
作者:
Steffen Schmitt;Maximilian Wick;Christian Wouters;L. Ruwe;Isabelle Graf;J. Andert;N. Hansen;S. Pisc

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为了更好地了解水添加量作为发动机HCCI燃烧控制参数的适用性,研究了水喷射对异辛烷燃烧过程的影响。几个实验相结合,包括预混合的低压火焰,射流搅拌反应器(JSR)和活塞流反应器(PFR),都在大气压力下,和单缸研究发动机(SCRE)与任一异辛烷或罗恩98汽油操作。在层流预混异辛烷/O2/Ar火焰(当量比Φ=1.4,40 mbar)中测定了水的热效应,水的摩尔分数为0 ~ 0.22,其中水的加入使激光诱导荧光(LIF)测量的温度降低了110 K。从这些火焰以及JSR(Φ=0.65,933 mbar)和PFR实验(Φ=0.65,970 mbar)中获得了在700-1100 K的低至中温范围内添加和不添加H2O的形态数据。在这些火焰和反应器实验中的化学分析是使用分子束质谱法(MBMS),采用电子电离(EI)的PFR和预混火焰或单光子电离(PI)的可调真空紫外辐射的JSR。对物种摩尔分数的影响是小的,这是支持从化学动力学模拟预测。利用傅里叶变换红外光谱(FTIR)获得了SCRE废气的定量形态数据。在实验室规模的实验和发动机运行中检测到非常相似的物种库。因此,假设这些结果可以帮助指导基本化学动力学以及HCCI发动机控制模型的改进。
The effect of H2O injection on the combustion process ofiso-octane was investigated with the aim to better understand the suitability of water addition as a potential engine control parameter for homogeneous-charge compression ignition (HCCI) combustion. Several experiments were combined including premixed low-pressure flames, a jet-stirred reactor (JSR) and a plug-flow reactor (PFR), both at atmospheric pressure, and a single-cylinder research engine (SCRE) operated with eitheriso-octane or RON 98 gasoline. The thermal effect of H2O addition was determined in laminar premixediso-octane/O2/Ar flames (equivalence ratio Φ=1.4, 40 mbar) with H2O mole fractions of 0 to 0.22, where water addition reduced the temperature measured by laser-induced fluorescence (LIF) by up to 110 K. Speciation data were obtained from these flames as well as in the JSR (Φ=0.65, 933 mbar) and PFR experiments (Φ=0.65, 970 mbar) with and without H2O addition in the low- to intermediate temperature regime from 700–1100 K. The chemical analysis in these flame and reactor experiments was performed using molecular-beam mass spectrometry (MBMS) employing either electron ionization (EI) in the PFR and premixed flame or single-photon ionization (PI) by tunable vacuum-ultraviolet radiation in the JSR. The effects on species mole fractions were small which is supported by predictions from chemical-kinetic simulations. Quantitative speciation data of the exhaust gas of the SCRE were obtained by using Fourier-transform infrared (FTIR) spectroscopy. A very similar species pool was detected in the laboratory-scale experiments and for the engine operation. It is thus assumed that these results could assist in guiding both the improvement of fundamental chemical-kinetic as well as HCCI engine control models.