Electrodynamic response of incoherent metals : Normal phase of iron pnictides

Electrodynamic response of incoherent metals : Normal phase of iron pnictides
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DOI:
10.1103/physrevb.79.024515
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发表时间:
2009-01
期刊:
影响因子:
3.7
通讯作者:
M. Laad;L. Craco;S. Leoni;H. Rosner
M. Laad;L. Craco;S. Leoni;H. Rosner
中科院分区:
物理与天体物理2区
文献类型:
--
作者:
M. Laad;L. Craco;S. Leoni;H. Rosner

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Received 9 October 2008; revised manuscript received 2 December 2008; published 22 January 2009 The recent discovery of high-temperature superconductivity in doped iron pnictides is the latest example of unanticipated behavior exhibited by d- and f-band materials. The symmetry of the superconductor SC gap, along with the mechanism of its emergence from the “normal” state, is a central issue in this context. Here, motivated by a host of experimental signatures suggesting strong correlations in the Fe pnictides, we undertake a detailed study of their normal state. Focusing on symmetry-unbroken phases, we use the correlated bandstructure method, local density approximation plus dynamical mean-field theory LDA+ DMFT, to study the one-particle responses of both LaO1�xFeAsFx and SmO1�xFeAsFx in detail. Basing ourselves on excellent quantitative agreement between LDA+ DMFT and key experiments probing the one-particle responses, we extend our study, undertaking the first detailed study of their normal-state electrodynamic response. In particular, we propose that near-total normal-state incoherence, resulting from strong, local correlations in the Fe d shell in Fe pnictides, underpins the incoherent normal-state transport found in these materials, and discuss the specific electronic mechanisms leading to such behavior. We also discuss the implications of our work for the multiband nature of the SC by studying the pairing “glue” function, which we find to be an overdamped electronic continuum. Similarities and differences between cuprates and Fe pnictides are also touched upon. Our study supports the view that SC in Fe pnictides arises from a bad-metallic incoherent “normal” state that is proximate to a Mott insulator.