Control of Product Distribution of Fischer–Tropsch Synthesis with a Novel Rotating Packed-Bed Reactor: From Diesel to Light Olefin
Control of Product Distribution of Fischer–Tropsch Synthesis with a Novel Rotating Packed-Bed Reactor: From Diesel to Light Olefin
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DOI：
10.1021/ie300079j
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发表时间：
2012-06
影响因子：
4.2
通讯作者：
Jianfeng Chen;Yi Liu;Yi Zhang
中科院分区：
文献类型：
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作者：
Jianfeng Chen;Yi Liu;Yi Zhang
首次将旋转填充床反应器应用于费托合成反应。通过选择最佳的超重力水平，可以选择性地形成FTS的主要产物，这为FTS的产物分布调节打开了一扇大门。RPB反应器中低碳烯烃的高选择性为合成气直接高效合成低碳烯烃、合成气制烯烃（STO）提供了新的途径，避免了低效率的甲醇合成和甲醇制烯烃（MTO）工艺。
A rotating packed-bed (RPB) reactor has been first applied to the Fischer–Tropsch synthesis (FTS) reaction. The main products of the FTS can be selectively formed by choosing the optimum high gravity level of the RPB reactor, which has opened a door to tailor the product distribution of FTS. The high selectivity of light olefins in RPB reactor provides a novel pathway to directly and effectively form light olefins from syngas, syngas to olefin (STO), which would avoid low-efficiency methanol synthesis and methanol-to-olefin (MTO) process.