CO2 capture cost saving through waste heat recovery using transport membrane condenser in different solvent-based carbon capture processes

CO2 capture cost saving through waste heat recovery using transport membrane condenser in different solvent-based carbon capture processes
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在不同溶剂型碳捕集工艺中使用传输膜冷凝器进行废热回收,从而节省二氧化碳捕集成本

DOI:
10.1016/j.energy.2020.119225
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发表时间:
2020-11
期刊:
影响因子:
9
通讯作者:
Shuiping Yan
Shuiping Yan
中科院分区:
工程技术1区
文献类型:
--
作者:
Qiufang Cui;Te Tu;Long Ji;Shuiping Yan

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采用传输膜冷凝器(TMC)对单乙醇胺(MEA)、二乙醇胺(DEA)、哌嗪(PZ)和甘氨酸钾(PG)富分流改进型碳捕集工艺中的热汽提气余热进行回收。220 h试验表明,TMC具有良好的余热回收性能稳定性。基于PZ的TMC改进的富分流工艺(即,PZ-case)实现了最高的废热回收性能,其次是PG-case、MEA-case和DEA-case。在废热回收过程中,热通量和水通量之间存在很强的线性关系。考虑了三种情景,以比较4种情况下的CO2捕获成本节约。当TMC面积固定时,即富气分流改造的额外投资相同时,PZ方案获得的CO2捕集成本节约最高(6.40美元/t-CO2),其次是PG方案、MEA方案和DEA方案。当需要600 kJ/kg-CO2的固定废热回收性能来获得相同的收益时,在富分流改造后,PZ-和PG-情况获得了相同的CO2捕获成本节省4.22美元/t-CO2。此外,当再沸器负荷降低潜力为15%时,PG-情况实现了最大的CO2捕集成本节约($4.56/t-CO2)。
In this study, the waste heat from the hot stripping gas was recovered by adopting the transport membrane condenser (TMC) in the monoethanolamine (MEA)-, diethanolamine (DEA)-, piperazine (PZ)- and potassium glycinate (PG)-based rich-split modified carbon capture processes. A 220-h test showed that TMC can exhibit a good stability on the waste heat recovery performance. The PZ-based TMC-modified rich-split process (i.e., PZ-case) achieved a highest waste heat recovery performance, followed by the PG-case, MEA-case and DEA-case. A strong linear relationship between the heat and water fluxes was observed during the waste heat recovery. Three scenarios were considered for comparing the CO2capture cost savings of 4 cases. When the TMC area was fixed meaning the same additional investment of rich-split modification, PZ-case gained the highest CO2capture cost saving ($6.40/t-CO2), followed by PG-, MEA- and DEA-case. When a fixed waste heat recovery performance of 600 kJ/kg-CO2was required for obtaining the same revenue after rich-split modification, PZ- and PG-case obtained the same CO2capture cost saving of $4.22/t-CO2. Moreover, when the reboiler duty reduction potential was aimed at 15%, PG-case achieved the maximum CO2capture cost saving ($4.56/t-CO2).
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