Roll coated large area ITO- and vacuum-free all organic solar cells from diketopyrrolopyrrole based non-fullerene acceptors with molecular geometry effects
Roll coated large area ITO- and vacuum-free all organic solar cells from diketopyrrolopyrrole based non-fullerene acceptors with molecular geometry effects
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由具有分子几何效应的二酮吡咯并吡咯基非富勒烯受体制成的辊涂大面积 ITO 和无真空全有机太阳能电池
DOI:
10.1039/c6ra06898g
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发表时间:
2016-04
期刊:
影响因子:
3.9
通讯作者:
Yu Donghong
中科院分区:
文献类型:
--
作者:
Br;t Rasmus Guldbaek;Zhang Fei;Andersen Thomas Rieks;Angmo Dechan;Shi Minmin;Gurevich Leonid;Krebs Frederik C.;Andreasen Jens Wenzel;Yu Donghong
In this paper, we investigate three diketopyrrolopyrrole (DPP) based small molecular non-fullerene acceptors, namely Ph(DPP)3, Ph(DPP)2, and PhDMe(DPP)2, focusing on molecular geometry effects on the frontier orbital level, light absorption, molecular configuration, electron mobility, thin film morphology, and photovoltaic performance of both spin-coated ITO based and roll coated large area, ITO- and vacuum-free organic solar cells (OSCs). For spin-coated devices based on P3HT as the donor polymer the solar cells gave power conversion efficiencies (PCEs) in the following order for (P3HT:PhDMe(DPP)2, 0.65%) > (P3HT:Ph(DPP)2, 0.48%) > (P3HT:Ph(DPP)3, 0.31%). All devices present an open circuit voltage (Voc) higher than 1.0 V. For the roll-coated devices, the PCEs were found to fall in another order and with lower values (P3HT:Ph(DPP)3, 0.54%) > (P3HT:Ph(DPP)2, 0.43%) > (P3HT:PhDMe(DPP)2, 0.04%) and the highest Voc was 0.82 V. Our preliminary results highlight the influence of geometry, structure and processing on the performance of non-fullerene acceptors.
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DOI:
10.1039/c5cp02800k
发表时间:
2015-06
期刊:
Physical chemistry chemical physics : PCCP
影响因子:
--
作者:
G. Dutton;S. Robey
通讯作者:
G. Dutton;S. Robey
影响因子:
3.3
作者:
Jin-Liang Wang;Zhicai He;Hongbin Wu;Yong Cao;J. Pei
通讯作者:
Jin-Liang Wang;Zhicai He;Hongbin Wu;Yong Cao;J. Pei
DOI:
10.1002/asia.201500476
发表时间:
2015
期刊:
Chem Asian J
影响因子:
--
作者:
Wei Huan;Chen Weichao;Han Liangliang;Wang Ting;Bao Xichang;Li Xiaoyun;Liu Jie;Zhou Yuanhang;Yang Renqiang
通讯作者:
Yang Renqiang
影响因子:
6.9
作者:
Krebs, Frederik C.
通讯作者:
Krebs, Frederik C.
影响因子:
4.4
作者:
Zhang Fei;Br;t Rasmus Guldbaek;Gu Zhuowei;Wu Shasha;Andersen Thomas Rieks;Shi Minmin;Yu Donghong;Chen Hongzheng
通讯作者:
Chen Hongzheng