Spin-Dynamics in Vicinity of Spin-Gap Phase Transition for Organic Conductor(TMTTF)_2X

Spin-Dynamics in Vicinity of Spin-Gap Phase Transition for Organic Conductor(TMTTF)_2X
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有机导体自旋间隙相变附近的自旋动力学(TMTTF)_2X

DOI:
10.1143/jpsj.79.043702
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发表时间:
2010
期刊:
J. Phys. Soc. Jpn.
影响因子:
--
通讯作者:
and T. Nakamura
and T. Nakamura
中科院分区:
--
文献类型:
--
作者:
K. Furukawa;T. Hara;and T. Nakamura

文献摘要

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通过脉冲 ESR 光谱研究了有机导体 (TMTTF)2PF6 的自旋间隙相变附近的自旋动力学。在基态和高温相之间的中间区域观察到弛豫时间的异常,并且与源自横向磁相互作用的电荷重新取向相关。重叠积分的计算意味着相当多的链间相互作用。横向磁相互作用在(TMTTF)2PF6 中的自旋能隙相变中起着重要作用。
The spin dynamics in the vicinity of the spin-gap phase transition for the organic conductor (TMTTF)2PF6were examined by pulsed-ESR spectroscopy. An anomaly in the relaxation time was observed in this intermediate region between the ground state and the high-temperature phase and was associated with the charge re-orientation originating in the transverse magnetic interaction. The calculation of the overlap integrals implied considerable inter-chain interactions. The transverse magnetic interaction plays an important role of the spin-gap phase transition in (TMTTF)2PF6.