Non-local real-space analysis of chiral optical signals.

Non-local real-space analysis of chiral optical signals.
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DOI:
10.1039/c6sc01743f
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发表时间:
2016-11-01
期刊:
影响因子:
8.4
通讯作者:
Mukamel S
Mukamel S
中科院分区:
化学1区
文献类型:
--
作者:
Rouxel JR;Chernyak VY;Mukamel S

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开发了线性手性信号(例如圆二色性)的空间非局部响应张量描述。开发了线性手性信号(例如圆二色性)的空间非局部响应张量描述。通过直接使用矢量势而不是电场和磁场,我们根据电荷和电流密度的相关函数重新构建信号,并避免了繁琐的多极展开。
A spatially non-local response tensor description of linear chiral signals such as circular dichroism is developed. A spatially non-local response tensor description of linear chiral signals such as circular dichroism is developed. By working directly with the vector potential rather that the electric and magnetic fields, we recast the signals in terms of correlation functions of charge and current densities and avoid the tedious expansion in multipoles.