Quantum coherence in molecular photoionization.
Quantum coherence in molecular photoionization.
复制标题
分子光电离中的量子相干性。
DOI：
10.1039/d2cp01562e
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发表时间：
2022
期刊：
影响因子：
--
通讯作者：
Ruberti M
中科院分区：
文献类型：
--
作者：
Ruberti M
研究多电子系统中超快量子相干的发生、衰减以及控制是阿秒物理的研究热点。对探测超快量子相干性的阿秒实验的解释需要应用先进的理论和计算工具，结合多电子理论，电子连续谱的描述，包括在强激光场的情况下，以及核动力学理论。本文综述了光电离分子系统中量子相干性的阿秒动力学理论研究进展，并概述了阿秒体系中相干性和纠缠的理论和实验研究的未来方向。
The study of onset and decay, as well as control of ultrafast quantum coherence in many-electron systems is in the focus of interest of attosecond physics. Interpretation of attosecond experiments detecting the ultrafast quantum coherence requires application of advanced theoretical and computational tools combining many-electron theory, description of the electronic continuum, including in the strong laser field scenario, as well as nuclear dynamics theory. This perspective reviews the recent theoretical advances in understanding the attosecond dynamics of quantum coherence in photoionized molecular systems and outlines possible future directions of theoretical and experimental study of coherence and entanglement in the attosecond regime.