Anthropogenic aerosols observed in Asian continental outflow at Jeju Island, Korea, in spring 2005
Anthropogenic aerosols observed in Asian continental outflow at Jeju Island, Korea, in spring 2005
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DOI：
10.1029/2008jd010306
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发表时间：
2009-02
影响因子：
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通讯作者：
L. Sahu;Y. Kondo;Y. Miyazaki;M. Kuwata;M. Koike;N. Takegawa;H. Tanimoto;H. Matsueda;Soon-chang Yoon;Young-Joon Kim
中科院分区：
文献类型：
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作者：
L. Sahu;Y. Kondo;Y. Miyazaki;M. Kuwata;M. Koike;N. Takegawa;H. Tanimoto;H. Matsueda;Soon-chang Yoon;Young-Joon Kim
（硫酸根）气溶胶分别为1.2±0.8毫克碳/立方米、4.2±1.6毫克碳/立方米、1.3±1.0毫克碳/立方米和4.0±3.4微克/立方米。几乎所有物质的浓度在中国气团中最高，而在海洋气团中最低。在中国流出气流中观测到的黑碳/二氧化碳斜率为9.7纳克/立方米·ppbv⁻¹，与中国东北地区黑碳/一氧化碳排放比的估计值相当合理地吻合。根据观测到的硫氧化物 - 一氧化碳相关性，计算出硫氧化物（二氧化硫 + 硫酸根）的传输效率为40 - 45%。硫酸根/黑碳和水溶性有机碳/黑碳的比率与从大陆传输时间的关系表明，大部分硫酸根和水溶性有机碳气溶胶是由大约……形成的
(SO4� ) aerosols were 1.2 ± 0.8 mgC m � 3 , 4.2 ± 1.6 mgC m � 3 , 1.3 ± 1.0 mgC m � 3 , and 4.0 ± 3.4 m gm � 3 , respectively. Almost all species concentrations were highest in Chinese air masses, while they were lowest in marine air masses. The observed DBC/DCO slope of 9.7 ng m � 3 ppbv � 1 in Chinese outflow agrees reasonably with the estimates of the BC/CO emission ratios over northeastern China. The transport efficiencies of SOx (SO2 +S O4� ) are calculated to be 40–45% from the observed SOx-CO correlation. The relationships of the SO4� /BC and WSOC/BC ratios with transport time from the continent suggest that a majority of SO4� and WSOC aerosols were formed by about