A Review on Halide Perovskite-Based Photocatalysts: Key Factors and Challenges.
A Review on Halide Perovskite-Based Photocatalysts: Key Factors and Challenges.
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DOI：
10.1021/acsaem.2c02680
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发表时间：
2022-12-26
影响因子：
6.4
通讯作者：
Eslava, Salvador
中科院分区：
文献类型：
--
作者：
Temerov, Filipp;Baghdadi, Yasmine;Rattner, Ed;Eslava, Salvador
关键词：
关于卤化物钙钛矿材料用于光催化反应的研究文章越来越多。这些文章将这些材料的巨大成功从太阳能电池扩展到光催化技术，如制氢、二氧化碳还原、染料降解和有机合成。在这篇综述文章中，我们首先描述了光催化的背景理论，然后描述了卤化物钙钛矿的性质及其在光催化方面的研究进展。我们重点介绍了影响其光催化性能的关键内在因素，如稳定性、电子能带结构和吸附性能。我们还讨论并阐明了它们在光催化中发展的关键考虑因素和挑战，如与反应条件、反应器设计、可降解有机物的存在和表征有关的问题，特别是在CO2光催化还原方面。通过对卤化物钙钛矿型光催化剂的综述，将为其合理的设计和开发提供更好的认识，并有助于其在光催化太阳能器件的广泛领域中的科学技术应用。
A growing number of research articles have been published on the use of halide perovskite materials for photocatalytic reactions. These articles extend these materials’ great success from solar cells to photocatalytic technologies such as hydrogen production, CO2 reduction, dye degradation, and organic synthesis. In the present review article, we first describe the background theory of photocatalysis, followed by a description on the properties of halide perovskites and their development for photocatalysis. We highlight key intrinsic factors influencing their photocatalytic performance, such as stability, electronic band structure, and sorption properties. We also discuss and shed light on key considerations and challenges for their development in photocatalysis, such as those related to reaction conditions, reactor design, presence of degradable organic species, and characterization, especially for CO2 photocatalytic reduction. This review on halide perovskite photocatalysts will provide a better understanding for their rational design and development and contribute to their scientific and technological adoption in the wide field of photocatalytic solar devices.
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