Nature does not rely on long-lived electronic quantum coherence for photosynthetic energy transfer

Nature does not rely on long-lived electronic quantum coherence for photosynthetic energy transfer
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DOI:
10.1073/pnas.1702261114
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发表时间:
2017-08-08
影响因子:
11.1
通讯作者:
Miller, R. J. Dwayne
Miller, R. J. Dwayne
中科院分区:
综合性期刊1区
文献类型:
--
作者:
Duan, Hong-Guang;Prokhorenko, Valentyn I.;Miller, R. J. Dwayne

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在光合作用的第一步,撞击太阳光子的能量转化为收集光的生物分子复合物的电子激发能。随后的能量转移到反应中心通常被合理地解释为激子在典型的时间尺度上在生物分子发色团网格上移动
During the first steps of photosynthesis, the energy of impinging solar photons is transformed into electronic excitation energy of the light-harvesting biomolecular complexes. The subsequent energy transfer to the reaction center is commonly rationalized in terms of excitons moving on a grid of biomolecular chromophores on typical timescales