Oxygen-Free Conversion of Methane to Ethylene in a Plasma-Followed-by-Catalyst (PFC) Reactor
Oxygen-Free Conversion of Methane to Ethylene in a Plasma-Followed-by-Catalyst (PFC) Reactor
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在等离子体催化 (PFC) 反应器中将甲烷无氧转化为乙烯
DOI：
10.1088/1009-0630/10/5/15
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发表时间：
2008-10
影响因子：
1.7
通讯作者：
Zhu Aimin
中科院分区：
文献类型：
--
作者：
Li Xiaosong;Wang Hui;Shi Chuan;Xu Yong;Wang Kangjun;Zhu Aimin
Oxygen-free conversion of methane to ethylene was investigated in a two-stage plasma-followed-by-catalyst (PFC) reactor. In the absence of catalyst, pulsed spark discharges and pulsed corona discharges were compared for methane conversion. The results showed that methane was mainly converted to acetylene, but pulsed spark discharges exhibited distinct advantages over the pulsed corona discharges in methane conversion. Thereby, pulsed spark discharges were employed and followed by Ag-Pd/SiO2 catalyst for achieving ethylene as a target product in the PFC reactor. Using the PFC reactor, a steady single-pass ethylene yield of 57% was obtained at a rate of methane conversion of 74%.
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