High yield of self-catalyzed GaAs nanowire arrays grown on silicon via gallium droplet positioning

High yield of self-catalyzed GaAs nanowire arrays grown on silicon via gallium droplet positioning
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DOI:
10.1088/0957-4484/22/27/275602
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发表时间:
2011-07-08
期刊:
影响因子:
3.5
通讯作者:
Caroff, P.
Caroff, P.
中科院分区:
材料科学3区
文献类型:
--
作者:
Plissard, S.;Larrieu, G.;Caroff, P.

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我们报告和详细的方法来实现垂直的自催化GaAs纳米线直接在Si(111)上的生长与接近完美的垂直产量,使用电子束定义的孔阵列在介电层和分子束外延。在我们的条件下,GaAs纳米线生长沿着气-液-固机制,使用原位自形成的Ga液滴。本文的重点是了解的作用,基板的准备和预生长条件。在不改变温度或V/III比的情况下,垂直纳米线的产率逐渐增加至95%。证明了实现非常密集的阵列的可能性,中心到中心的线间距离小于100 nm。
We report and detail a method to achieve growth of vertical self-catalyzed GaAs nanowires directly on Si(111) with a near-perfect vertical yield, using electron-beam-defined arrays of holes in a dielectric layer and molecular beam epitaxy. In our conditions, GaAs nanowires are grown along a vapor-liquid-solid mechanism, using in situ self-forming Ga droplets. The focus of this paper is to understand the role of the substrate preparation and of the pre-growth conditioning. Without changing temperature or the V/III ratio, the yield of vertical nanowires is increased incrementally up to 95%. The possibility to achieve very dense arrays, with center-to-center inter-wire distances less than 100 nm, is demonstrated.