Magnetoelectric effect in the quantum spin gap system TlCuCl3
Magnetoelectric effect in the quantum spin gap system TlCuCl3
复制标题
量子自旋间隙系统 TlCuCl3 中的磁电效应
DOI:
10.1103/physrevb.95.184420
复制
发表时间:
2017
影响因子:
3.7
通讯作者:
and H. Tanaka
中科院分区:
文献类型:
--
作者:
S. Kimura;K. Kakihata;Y. Sawada;K. Watanabe;M. Matsumoto;M. Hagiwara;and H. Tanaka
Quantum magnets, which involve strong quantum fluctuation stemming from noncommutative properties of spin operators, have attracted much attention because of those fascinating properties. In this paper, we report detailed behaviors of the ferroelectricity, driven by the field-induced Bose-Einstein condensation of magnon quasiparticles in the quantum spin gap system. Superposition of the wave functions inherent in a quantum magnet in its ground state plays a key role in the appearance of this ferroelectricity. The field dependence of the spontaneous electric polarization clearly demonstrates that the ferroelectricity is caused by the emergence of the vector spin chirality in the magnon Bose-Einstein condensate. The ferroelectricity is suggested to be significantly enhanced by quantum entanglement in the spin dimer. Furthermore, reflecting the isotropic nature of, the ferroelectricity is very soft with a low electric coercive fieldMV/m. Our analysis indicates that vector components of the electric polarization, which are not caused by the spin current mechanism, appear in.