Probing Active-Site Relocation in Cu/SSZ-13 SCR Catalysts during Hydrothermal Aging by In Situ EPR Spectroscopy, Kinetics Studies, and DFT Calculations

Probing Active-Site Relocation in Cu/SSZ-13 SCR Catalysts during Hydrothermal Aging by In Situ EPR Spectroscopy, Kinetics Studies, and DFT Calculations
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DOI：
10.1021/acscatal.0c01590
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发表时间：
2020-06
期刊：
ACS Catalysis
影响因子：
12.9
通讯作者：
Yani Zhang;Yue Peng;Junhua Li;Kyle Groden;Jean-Sabin McEwen;E. Walter;Ying Chen;Yong Wang;F. Gao
Yani Zhang;Yue Peng;Junhua Li;Kyle Groden;Jean-Sabin McEwen;E. Walter;Ying Chen;Yong Wang;F. Gao
中科院分区：
化学1区
文献类型：
--
作者：
Yani Zhang;Yue Peng;Junhua Li;Kyle Groden;Jean-Sabin McEwen;E. Walter;Ying Chen;Yong Wang;F. Gao

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Cu/SSZ-13选择性催化还原催化剂在温和的水热老化后表现出活性损失，没有载体降解或孤立铜阳离子含量的损失。通过施加电子参数。
Cu/SSZ-13 selective catalytic reduction catalysts display activity loss after mild hydrothermal aging without support degradation or loss of isolated Cu cation content. By applying electron paramag...