Determination of the Fermi velocity by angle-dependent periodic orbit resonance measurements in the organic conductor α − ( BEDT − TTF ) 2 KHg ( SCN ) 4
Determination of the Fermi velocity by angle-dependent periodic orbit resonance measurements in the organic conductor α − ( BEDT − TTF ) 2 KHg ( SCN ) 4
复制标题
通过有机导体中与角度相关的周期轨道共振测量来确定费米速度 α − ( BEDT − TTF ) 2 KHg ( SCN ) 4
DOI:
10.1103/physrevb.66.134513
复制
发表时间:
2002
影响因子:
3.7
通讯作者:
J. Qualls
中科院分区:
文献类型:
--
作者:
A. Kovalev;S. Hill;J. Qualls
We report on detailed angle-dependent studies of the microwave $(\ensuremath{\nu}=50\char21{}90\mathrm{GHz})$ interlayer magnetoelectrodynamics of a single crystal sample of the organic charge-density-wave (CDW) conductor $\ensuremath{\alpha}\ensuremath{-}(\mathrm{BEDT}\ensuremath{-}\mathrm{TTF}{)}_{2}\mathrm{KHg}(\mathrm{SCN}{)}_{4}.$ Recently developed instrumentation enables both magnetic-field $(\mathbf{B})$ sweeps for a fixed sample orientation and angle sweeps at fixed $\ensuremath{\nu}/\mathbf{B}.$ We observe series' of resonant absorptions, which we attribute to periodic orbit resonances (POR)\char22{}a phenomenon closely related to cyclotron resonance. The angle dependence of the POR indicates that they are associated with the low-temperature quasi-one-dimensional (Q1D) Fermi surface (FS) of the title compound; indeed, all of the resonance peaks collapse onto a single set of $\ensuremath{\nu}/\mathbf{B}$ versus angle curves, generated using a semiclassical magnetotransport theory for a single Q1D FS. We show that Q1D POR measurements provide one of the most direct methods for determining the Fermi velocity, without any detailed assumptions concerning the band structure; our analysis yields an average value of ${v}_{F}=6.5\ifmmode\times\else\texttimes\fi{}{10}^{4}\mathrm{m}/\mathrm{s}.$ Quantitative analysis of the POR harmonic content indicates that the Q1D FS is strongly corrugated. This is consistent with the assumption that the low-temperature FS derives from a reconstruction of the high-temperature quasi-two-dimensional FS, caused by the CDW instability. Detailed analysis of the angle dependence of the POR yields parameters associated with the CDW superstructure, which are consistent with published results. Finally, we address the issue as to whether or not the interlayer electrodynamics are coherent in the title compound. We obtain a relaxation time from the POR linewidths, which is considerably longer than the interlayer hopping time, indicating that the transport in this direction is coherent.
DOI:
--
发表时间:
2019
期刊:
千葉大学ユーラシア言語文化論集
影响因子:
--
作者:
Keiichi Tajima;Mafuyu Kitahara;and Kiyoko Yoneyama;吉本啓;田口善久
通讯作者:
田口善久