A general dissolution-recrystallization strategy to achieve sulfur-encapsulated carbon for an advanced lithium-sulfur battery
A general dissolution-recrystallization strategy to achieve sulfur-encapsulated carbon for an advanced lithium-sulfur battery
复制标题
用于先进锂硫电池的硫包封碳的通用溶解-重结晶策略
DOI：
10.1039/c8ta02180e
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发表时间：
2018-07-07
影响因子：
11.9
通讯作者：
Mai, Kancheng
中科院分区：
文献类型：
--
作者：
Fan, Xuliang;Zhang, Yangfan;Mai, Kancheng
Herein, a general strategy is first proposed to fabricate a class of carbon@S cathodes via dissolution recrystallization of granular sulfur into a uniformsulfur layer-encapsulated carbon in a selective solution, guided by density functional theory calculations and the mechanism of crystal nucleation and growth. Significantly, all the carbon@S (SWNT@S, MWNT@S, and YP80@S) cathodes deliver superior rate performance and good cyclic durability. Furthermore, a flexible pouch Li-S battery, assembled based on a free-standing SWNT@S film, was demonstrated with good mechanical properties and deformation durability.
