Effect of overlying water pH, temperature, and hydraulic disturbance on heavy metal and nutrient release from drinking water reservoir sediments

Effect of overlying water pH, temperature, and hydraulic disturbance on heavy metal and nutrient release from drinking water reservoir sediments
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上覆水 pH 值、温度和水力扰动对饮用水水库沉积物重金属和营养物释放的影响

DOI:
10.1002/wer.1587
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发表时间:
2021-05
影响因子:
3.1
通讯作者:
Wang Xianyun
Wang Xianyun
中科院分区:
环境科学与生态学4区
文献类型:
--
作者:
Peng Cheng;Huang Yunying;Yan Xuchen;Jiang Lei;Wu Xuefei;Zhang Wei;Wang Xianyun

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How environmental factors impact the release of pollutants from sediment is critical to ensure the safety of drinking water, especially when the seasons change. Here, we investigated the effect of water pH, temperature, and hydraulic disturbance on the release of heavy metals and nutrients from the sediment of drinking water reservoir. The results show that lower initial water pH promoted the Zn release, while low temperature enhanced the Mn flux after 15 days. Meanwhile, continuous disturbance caused more metals releasing from sediment than intermittent disturbance due to greater shear stress and turbulence effect. However, intermittent high‐speed disturbance greatly altered the dynamic release of Zn from L‐shaped curve to U‐shape in water column. Moreover, lower water pH caused higher ammonium in water but lower nitrate since H+ restrained the nitrification. Yet, higher temperature inhibited the release of ammonium from sediment, which might relate to the accelerated mineralization of organic nitrogen and elevated dissolved oxygen caused by the algae growth. Notably, hydraulic disturbance with various intensity and duration greatly influenced the fluxes of various species of nitrogen and soluble phosphate in water column, because the disturbance facilitated the nitrogen and phosphorus exchanges between sediment–water and water–air interfaces.
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