Decomposition of Perfluorooctanesulfonate ( PFOS ) by Multiple Alternating Argon Plasmas in Bubbles with Gas Circulation

Decomposition of Perfluorooctanesulfonate ( PFOS ) by Multiple Alternating Argon Plasmas in Bubbles with Gas Circulation
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气体循环气泡中多次交替氩等离子体分解全氟辛烷磺酸 ( PFOS )

DOI:
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发表时间:
2015
期刊:
--
影响因子:
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通讯作者:
K. Yasuoka
K. Yasuoka
中科院分区:
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文献类型:
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作者:
H. Obo;N. Takeuchi;K. Yasuoka

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Perfluorooctanesulfonate (PFOS) is used in a wide range of industrial applications, owing to its superior characteristics; however, its environmental persistence and biopersistence have become matters of concern, leading to the demand for decomposition treatments for industrial effluent containing PFOS. Although it is possible to decompose PFOS using direct current plasma generated within bubbles in water, low time and energy efficiencies arising from ballast resistance losses are major issues. This paper reports on the development of a reactor for generating plasma, with the number of treatment holes increased from one (in previous studies) to 21. Decomposition of 1 L of PFOS in 1200 min was successfully completed using this reactor, with a mass balance of fluorine reaching 90% or more over time. Furthermore, loss of ballast elements, which are used to stably generate electrical discharge, was significantly reduced by switching from resistors to capacitors. The exhaust gas from the reactor was recirculated through the treatment holes to successfully reduce the gas consumption flow rate to approximately 10% that of conventional systems. Keywords—Perfluorooctanesulfonates (PFOS), plasma, water treatment, organic fluorine Corresponding author: Hayato Obo e-mail address: hayato@obolab.com 62 International Journal of Plasma Environmental Science & Technology, Vol.9, No.1, APRIL 2015
DOI: 10.1021/es800832p
发表时间: 2008-10-01
影响因子: 11.4
作者:
Hori, Hisao;Nagaoka, Yumiko;Kutsuna, Shuzo
通讯作者: Kutsuna, Shuzo
DOI: 10.1021/es0484754
发表时间: 2005-04-01
影响因子: 11.4
作者:
Hori, H;Yamamoto, A;Kutsuna, S
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DOI: 10.1021/es049719n
发表时间: 2004-11-15
影响因子: 11.4
作者:
Hori, H;Hayakawa, E;Arakawa, R
通讯作者: Arakawa, R
水中气泡内的脉冲等离子体发展
DOI: --
发表时间: 2008
期刊:
影响因子: --
作者:
Koichi YASUOKA;and Keisuke SATO
通讯作者: and Keisuke SATO