Modulation of Photoinduced Transmembrane Currents in a Fullerene-Doped Freestanding Lipid Bilayer by a Lateral Bias

Modulation of Photoinduced Transmembrane Currents in a Fullerene-Doped Freestanding Lipid Bilayer by a Lateral Bias
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DOI:
10.1021/acsomega.9b02336
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发表时间:
2019-11-05
期刊:
影响因子:
4.1
通讯作者:
Hirano-Iwata, Ayumi
Hirano-Iwata, Ayumi
中科院分区:
化学3区
文献类型:
--
作者:
Ma, Teng;Feng, Xingyao;Hirano-Iwata, Ayumi

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我们报道了一种新的脂质双层系统,在该系统中,除了传统的跨膜电压外,还可以施加横向偏压。在微孔中形成了掺杂[6,6]-苯基-C-61-丁酸甲酯(PCBM)的独立双层脂膜(BLM),并在其周围沉积了金属电极。使用该系统,可以通过沿BLM施加横向偏置来调制和放大光诱导的跨膜电流。结果表明,埋入电极的微细硅片是形成基于PCBM掺杂BLM的类晶体管器件的良好平台,具有广泛的应用前景。
We report on a novel lipid bilayer system, in which a lateral bias can be applied in addition to a conventional transmembrane voltage. Freestanding bilayer lipid membranes (BLMs) doped with [6,6]-phenyl-C-61-butyric acid methyl ester (PCBM) were formed in a microaperture, around which metal electrodes were deposited. Using this system, it was possible to modulate and amplify photoinduced transmembrane currents by applying a lateral bias along the BLM. The results indicate that the microfabricated Si chip with embedded electrodes is a promising platform for the formation of transistor-like devices based on PCBM-doped BLMs and have potential for use in a wide variety of nanohybrid devices.