Facile synthesis of a high-performance titanosilicate catalyst with controllable defective Ti(OSi)3OH sites.
Facile synthesis of a high-performance titanosilicate catalyst with controllable defective Ti(OSi)3OH sites.
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DOI：
10.1039/c8cc02794c
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发表时间：
2018-06
影响因子：
4.9
通讯作者：
Lizhi Wu;Zhimou Tang;Yunkai Yu;Xuting Yao;Wei Liu;Li Li-Li;Bing‐Jie Yan;Yue M. Liu;M. He
中科院分区：
文献类型：
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作者：
Lizhi Wu;Zhimou Tang;Yunkai Yu;Xuting Yao;Wei Liu;Li Li-Li;Bing‐Jie Yan;Yue M. Liu;M. He
采用巧妙的策略构建了一种新缺陷Ti（OSi）3OH物种的TS-1（TS-1 S）催化剂，该物种在不同Ti物种中表现出最高的反应活性。这也提供了一种有前途的方式来有效地调整其他钛硅酸盐中的Ti活性中心的固有性质。
A novel TS-1 (TS-1S) catalyst with newly-generated defects, i.e. Ti(OSi)3OH species, which exhibits the highest reactivity among different Ti species, is constructed in an ingenious strategy. This also provides a promising way to effectively tune the intrinsic nature of Ti active centres in other titanosilicates.