Effect of tungsten deposition thickness on hydrogen isotope permeation through RAFM steel

Effect of tungsten deposition thickness on hydrogen isotope permeation through RAFM steel
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钨沉积厚度对 RAFM 钢氢同位素渗透的影响

DOI:
10.1016/j.jnucmat.2020.152647
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发表时间:
2020-11
影响因子:
3.1
通讯作者:
Guang-Nan Luo
Guang-Nan Luo
中科院分区:
工程技术2区
文献类型:
--
作者:
Hao-Dong Liu;Hai-Shan Zhou;Li Qiao;Hong Zhang;Guang-Nan Luo

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进行了氘等离子体驱动渗透(PDP)实验,通过减少激活铁素体/马氏体(RAFM)钢与无钨(W)沉积层。结果表明,W沉积并不总是作为D渗透阻挡层,但在一定条件下提高D渗透通量通过结构材料。在稳态下,PDP通过具有薄(~30 nm)W沉积层的RAFM钢的通量大于裸RAFM钢的通量,而具有厚(6.0 μm)W沉积层的RAFM钢膜的渗透通量低于裸钢样品的通量。氚迁移分析程序(TMAP)的计算表明,稳态渗透通量取决于W层与RAFM钢界面处累积的氚浓度,且与W层厚度密切相关。只有当W厚度大于~2 μm时,稳态渗透通量才由W沉积层中的扩散控制。
Deuterium (D) plasma-driven permeation (PDP) experiments through reduced activation ferritic/martensitic (RAFM) steel with and without tungsten (W) deposition layer have been performed. The results confirm that W deposition does not always work as D permeation barrier, but enhances D permeation flux through the structural material under certain conditions. The steady state PDP fluxes through RAFM steel with a thin (~30 nm) W deposition layer have been found to be larger than those of bare RAFM steel, whereas the RAFM steel membrane with a thick (6.0 μm) W deposition layer exhibits lower permeation fluxes than those of bare steel sample. Tritium Migration Analysis Program (TMAP) calculation indicates that the steady state permeation flux is determined by the D concentration accumulated at the interface between W layer and RAFM steel, which is highly relevant to the W deposition thickness. Only when the W thickness is larger than ~2 μm, the steady state permeation flux will be controlled by diffusion in W deposition layer.
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