Changes in deep Pacific circulation and carbon storage during the Pliocene-Pleistocene transition
Changes in deep Pacific circulation and carbon storage during the Pliocene-Pleistocene transition
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DOI:
10.1016/j.epsl.2023.118020
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发表时间:
2023-03
影响因子:
5.3
通讯作者:
Z. Jian;H. Dang;Jimin Yu;Qiong Wu;X. Gong;C. Stepanek;C. Colin;Lili Hu;G. Lohmann;Xiaoli Zhou;S. Wan
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文献类型:
--
作者:
Z. Jian;H. Dang;Jimin Yu;Qiong Wu;X. Gong;C. Stepanek;C. Colin;Lili Hu;G. Lohmann;Xiaoli Zhou;S. Wan
The global climate has been gradually cooling over the Cenozoic and is punctuated by the intensification of Northern Hemisphere Glaciation (NHG) from the latest Pliocene to earliest Pleistocene (∼3.1–2.5 millions of years ago, Ma). A decline of atmospheric CO2is supposed as a prerequisite for the NHG, but the associated carbon-cycle processes remain elusive. Here we combine foraminiferal records of neodymium isotope and boron-calcium ratio, and simulations of an Earth system model, to investigate changes in the water-mass composition and carbonate-ion concentration of the deep Pacific Ocean during the NHG. Our proxy records have revealed a significant expansion of southern-sourced waters with increased respired carbon storage into the deep Pacific during the NHG. These changes may be explained by strengthened deep-water formation and biological-pump efficiency in the Southern Ocean due to Antarctic sea-ice growth, as suggested by our model experiments and evidence from the Sub-Antarctic region. These results provide key clues for quantifying the role of the dissolved inorganic carbon content of deep Pacific waters in modulating atmospheric CO2during the NHG.