Self-supported tremella-like MoS2-AB particles on nickel foam as bifunctional electrocatalysts for overall water splitting

Self-supported tremella-like MoS2-AB particles on nickel foam as bifunctional electrocatalysts for overall water splitting
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DOI:
10.1016/j.nanoen.2021.106707
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发表时间:
2021-11-27
期刊:
影响因子:
17.6
通讯作者:
Liu, Yongsheng
Liu, Yongsheng
中科院分区:
材料科学1区
文献类型:
--
作者:
Guo, Lingyun;Liu, Qian;Liu, Yongsheng

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The technology of electrolytic water splitting to produce hydrogen is considered a promising method for renewable energy utilization. It is essential to develop bifunctional electrode materials with low cost and high activity. Herein, tremella-like MoS2-AB particles on nickel foam substrate were fabricated through a one-step Solvothermal reaction and exhibited excellent electrocatalytic performance for over-water electrolysis in alkaline media, i.e., overpotentials of 77 and 248 mV to achieve catalytic current density 10 mA cm-2 for hydrogen evolution reaction and oxygen evolution reaction, respectively. Moreover, the two-electrode device demanded 1.51 V cell voltage to reach 10 mA cm-2 and showed good stability of 12 h without iR compensation. This work may afford a new idea to design self-supported bifunctional electrocatalysts toward efficient overall water splitting reactions.