Recent Advances in Hydrotreating of Pyrolysis Bio-Oil and Its Oxygen-Containing Model Compounds
Recent Advances in Hydrotreating of Pyrolysis Bio-Oil and Its Oxygen-Containing Model Compounds
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DOI：
10.1021/cs400069z
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发表时间：
2013-04
期刊：
影响因子：
12.9
通讯作者：
Huamin Wang;J. Male;Yong Wang
中科院分区：
文献类型：
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作者：
Huamin Wang;J. Male;Yong Wang
世界范围内对发现可替代化石燃料的可再生能源存在相当大的兴趣。木质纤维素生物质是地球上最丰富和最便宜的可再生原料，具有可持续生产燃料，化学品和碳基材料的巨大潜力。与加氢处理集成的快速热解是将木质纤维素生物质转化为用于运输的液态烃燃料的最简单、最具成本效益和最有效的方法之一，近几十年来引起了极大的关注。然而，热解生物油的有效加氢处理对经由热解-加氢处理的生物质转化的商业化提出了严峻的挑战。具体地，由于目前热解生物油原料的质量差（即，高氧含量、分子复杂性、焦化倾向和腐蚀性）。已经进行了大量的研究，以...
Considerable worldwide interest exists in discovering renewable energy sources that can substitute for fossil fuels. Lignocellulosic biomass, the most abundant and inexpensive renewable feedstock on the planet, has a great potential for sustainable production of fuels, chemicals, and carbon-based materials. Fast pyrolysis integrated with hydrotreating, one of the simplest, most cost-effective, and most efficient processes to convert lignocellulosic biomass to liquid hydrocarbon fuels for transportation, has attracted significant attention in recent decades. However, effective hydrotreating of pyrolysis bio-oil presents a daunting challenge to the commercialization of biomass conversion via pyrolysis-hydrotreating. Specifically, the development of active, selective, and stable hydrotreating catalysts is problematic due to the poor quality of current pyrolysis bio-oil feedstock (i.e., high oxygen content, molecular complexity, coking propensity, and corrosiveness). Significant research has been conducted to...