Spin-reorientation transition of Ni/Cu(100) and CO/Ni/Cu(100): Separation of the surface and bulk components of the X-ray magnetic circular dichroism spectrum

Spin-reorientation transition of Ni/Cu(100) and CO/Ni/Cu(100): Separation of the surface and bulk components of the X-ray magnetic circular dichroism spectrum
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DOI:
10.1103/physrevb.71.214420
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发表时间:
2005-06-01
期刊:
影响因子:
3.7
通讯作者:
Yokoyama, T
Yokoyama, T
中科院分区:
物理与天体物理2区
文献类型:
--
作者:
Amemiya, K;Sakai, E;Yokoyama, T

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采用深度分辨X射线磁圆二色性(XMCD)技术研究了Ni/Cu(100)和CO/Ni/Cu(100)薄膜的自旋取向转变。分别提取表面层和内层的 XMCD 光谱。对于裸镍薄膜,表层的面内轨道磁矩显着增强。相反,内层表现出比面内层更大的垂直轨道磁矩。 CO 吸附后,表面磁化强度急剧降低,而内层不受影响。这些结果直接解释了 Ni/Cu(100) 和 CO/Ni/Cu(100) 中的自旋取向转变。
The spin-reorientation transition of Ni/Cu(100) and CO/Ni/Cu(100) films was investigated with the depth-resolved x-ray magnetic circular dichroism (XMCD) technique. The XMCD spectra from the surface and inner layers were separately extracted. As for the bare Ni films, the in-plane orbital magnetic moment in the surface layer is significantly enhanced. In contrast, the inner layers exhibit larger perpendicular orbital magnetic moment than the in-plane one. Upon CO adsorption, the surface magnetization is drastically reduced, while the inner layers are unaffected. These results directly explain the spin-reorientation transition in Ni/Cu(100) and CO/Ni/Cu(100).