Preparation of bulk AgNWs/PEDOT:PSS composites: a new model towards high-performance bulk organic thermoelectric materials

Preparation of bulk AgNWs/PEDOT:PSS composites: a new model towards high-performance bulk organic thermoelectric materials
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块状AgNWs/PEDOT:PSS复合材料的制备:高性能块状有机热电材料的新模型

DOI:
10.1039/c5ra05551b
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发表时间:
2015-05
期刊:
影响因子:
3.9
通讯作者:
Jiang Wan
Jiang Wan
中科院分区:
化学3区
文献类型:
--
作者:
Liu Yuan;Song Zijun;Zhang Qihao;Zhou Zhenxing;Tang Yijing;Wang Lianjun;Zhu Juanjuan;Luo Wei;Jiang Wan

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一个简单而有效的方法被证明是制备高性能的块体AgNW/PEDOT:PSS热电复合材料。详细研究了不同AgNW含量样品的热电性能。结果表明,AgNW在PEDOT:PSS中的良好分散可以在不降低Seebeck系数或增加热导率的情况下提高电导率,这表明实现了电导率和Seebeck系数的解耦和优化。因此,观察到最大ZT比纯PEDOT:PSS样品的最大ZT大340%。我们的工作清楚地证明,AgNW的引入是一个有前途的模型,以显着提高散装有机基热电材料的热电性能。
A facile and effective approach is demonstrated to prepare high-performance bulk AgNWs/PEDOT:PSS thermoelectric composites. The thermoelectric properties of the samples with different AgNWs contents are investigated in detail. The results show that well-dispersed AgNWs in the bulk PEDOT:PSS can give rise to a much higher electrical conductivity without a noticeable decrease in Seebeck coefficient or increase in thermal conductivity, which suggests the achievement of decoupling and optimizing the electrical conductivity and Seebeck coefficient. Consequently, the maximum ZT is observed to be 340% larger than that of the pure PEDOT:PSS sample. Our work clearly proves that the introduction of AgNWs is a promising model to significantly improve the thermoelectric properties of bulk organic-based TE materials.
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