Aerosol Jet Printed p- and n-type Electrolyte-Gated Transistors with a Variety of Electrode Materials: Exploring Practical Routes to Printed Electronics
Aerosol Jet Printed p- and n-type Electrolyte-Gated Transistors with a Variety of Electrode Materials: Exploring Practical Routes to Printed Electronics
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DOI：
10.1021/am504171u
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发表时间：
2014-11-12
影响因子：
9.5
通讯作者：
Frisbie, C. Daniel
中科院分区：
文献类型：
--
作者：
Hong, Kihyon;Kim, Se Hyun;Frisbie, C. Daniel
印刷电功能液体油墨是实现柔性电子电路低成本、大面积、添加剂制造的一种很有前途的方法。要打印薄膜晶体管(薄膜电子器件的基本组成部分)，重要的是要有几种可打印电极材料的选择，这些材料具有高导电性、高稳定性和低成本。在这里，我们报告了完全气溶胶喷印(AJP)p和n型电解质门控晶体管(EGTS)使用各种不同的电极材料，包括高导电金属纳米颗粒(银)，导电聚合物(聚苯乙烯-磺酸掺杂聚(3，4-乙二氧基噻吩基，PEDOT：PSS))，透明碳基材料(还原石墨烯氧化物)。使用这些源漏电极材料和PEDOT：PSS/离子凝胶栅堆栈，我们展示了与聚(3-己基噻吩基)和氧化锌半导体相结合的全印刷p和n型EGTS。所有晶体管组件(包括电极、半导体和栅极绝缘体)均由AJP印刷。这两种器件都表现出典型的p型和n型晶体管特性，并且都表现出低阈值电压(
Printing electrically functional liquid inks is a promising approach for achieving low-cost, large-area, additive manufacturing of flexible electronic circuits. To print thin-film transistors, a basic building block of thin-film electronics, it is important to have several options for printable electrode materials that exhibit high conductivity, high stability, and low-cost. Here we report completely aerosol jet printed (AJP) p- and n-type electrolyte-gated transistors (EGTs) using a variety of different electrode materials including highly conductive metal nanopartides (Ag), conducting polymers (polystyrene-sulfonate doped poly(3,4-ethylendedioxythiophene, PEDOT:PSS), transparent carbon-based materials (reduced graphene oxide). Using these source-drain electrode materials and a PEDOT:PSS/ion gel gate stack, we demonstrated all-printed p- and n-type EGTs in combination with poly(3-hexythiophene) and ZnO semiconductors. All transistor components (including electrodes, semiconductors, and gate insulators) were printed by AJP. Both kinds of devices showed typical p- and n-type transistor characteristics, and exhibited both low-threshold voltages (