Recent development on core-shell photo(electro)catalysts for elimination of organic compounds from pharmaceutical wastewater

Recent development on core-shell photo(electro)catalysts for elimination of organic compounds from pharmaceutical wastewater
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DOI:
10.1016/j.chemosphere.2022.134311
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发表时间:
2022-03-28
期刊:
影响因子:
8.8
通讯作者:
Maruthapillai, Arthanareeswari
Maruthapillai, Arthanareeswari
中科院分区:
环境科学与生态学2区
文献类型:
--
作者:
Balu, Surendar;Chuaicham, Chitiphon;Maruthapillai, Arthanareeswari

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药物有机物是当代人类研究的一个重要里程碑,因为它们治疗各种疾病,提高人类的生活质量。然而,随着生态系统中抗菌素耐药性(AMR)的大幅上升,这些有机化合物被认为是受孕后的主要环境危害之一。目前已有多种生物技术和催化技术来去除水体系中的这些有机物,但都有其局限性。高级氧化工艺(AOPS)通过产生高氧化电位的活性物种来分解废水中的这些药物有机化合物。综述了各种光催化剂和光催化氧化技术,特别是核壳材料在光(电)催化降解制药废水中的应用。详细介绍了核壳催化剂的设计和最新进展,比较了光催化、电催化和光电催化在制药废水处理中的应用。此外,还详细讨论了无机和有机核壳材料的混合物以及基于金属-有机骨架的核壳催化剂对抗生素降解的影响。
Pharmaceutical organics are a vital milestone in contemporary human research since they treat various diseases and improve the quality of human life. However, these organic compounds are considered one of the major environmental hazards after the conception, along with the massive rise in antimicrobial resistance (AMR) in an ecosystem. There are various biological and catalytic technologies existed to eliminate these organics in aqueous system with their limitation. Advanced Oxidation processes (AOPs) are used to decompose these pharmaceutical organic compounds in the wastewater by generating reactive species with high oxidation potential. This review focused various photocatalysts, and photocatalytic oxidation processes, especially core-shell materials for photo (electro)catalytic application in pharmaceutical wastewater decomposition. Moreover, we discussed in details about the design and recent developments of core shell catalysts and comparison for photocatalytic, electrocatalytic and photo electrocatalytic applications in pharmaceutical wastewater treatment. In addition, the mixture of inorganic and organic core-shell materials, and metal-organic framework-based core-shell catalysts discussed in detail for antibiotic degradation.