Modeling and analysis of solid catalyzed reactive HiGee stripping

Modeling and analysis of solid catalyzed reactive HiGee stripping
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DOI:
10.1016/j.ces.2012.06.008
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发表时间:
2012-10
影响因子:
4.7
通讯作者:
Krishna Gudena;G. P. Rangaiah;S. Lakshminarayanan
Krishna Gudena;G. P. Rangaiah;S. Lakshminarayanan
中科院分区:
工程技术2区
文献类型:
--
作者:
Krishna Gudena;G. P. Rangaiah;S. Lakshminarayanan

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Increasing emphasis on process intensification for enhancing industrial chemical processes opens up many promising opportunities for an integrated rather than sequential (the onion-model approach) process synthesis and design. The present article introduces the concept of solid catalyzed reactive HiGee stripper (SCRHS) where reaction and stripping are integrated in a solid catalytic rotating packed bed. SCRHS is modeled for an esterification reaction, and analyzed in detail. Rotation of reactive stripper offers several advantages such as faster mass-transfer and higher product concentration over conventional reactors. Intraparticle diffusion-based modeling, component-based effectiveness factor, and instantaneous selectivity provide several insights into the proposed integrated process. Obtained results are encouraging and show that SCRHS is a promising candidate for future esterification plants.