Paper-based thermoelectric generator based on multi-walled carbon nanotube/carboxylated nanocellulose

Paper-based thermoelectric generator based on multi-walled carbon nanotube/carboxylated nanocellulose
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DOI:
10.1016/j.jpowsour.2021.229992
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发表时间:
2021-05-11
影响因子:
9.2
通讯作者:
Li, Xia
Li, Xia
中科院分区:
工程技术2区
文献类型:
--
作者:
Li, Hongbing;Zong, Yudong;Li, Xia

文献摘要

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Cellulose is the most abundant polymer material in nature. After being produced on the nanometer scale, it is widely used in research on flexible energy storage equipment and power supply equipment. Therefore, this study has prepared a nanocomposite thermoelectric material based on multi-walled carbon nanotube (MWCNT) and carboxylated nanocellulose fiber (C-CNF) and obtained a free-standing paper-based thermoelectric generator (TEG) through a simple printing method. The equipment exhibits excellent mechanical flexibility. At the same time, the thermal conductivity is significantly reduced under the dual effects of paper and C-CNF (is reduced to 0.02-0.09 W/mK). The TEG prototype has four P-shaped feet. Under a temperature gradient of 70 K, the open circuit voltage is 3.3 mV, and the output power is up to 3.7 nW. This work not only confirms the improvement of MWCNT thermoelectric performance by C-CNF but also provides a new strategy for the preparation of low-cost and environmentally friendly thermoelectric generators.