Current vs Charge Density Contributions to Nonlinear X-ray Spectroscopy.

Current vs Charge Density Contributions to Nonlinear X-ray Spectroscopy.
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电流与电荷密度对非线性 X 射线光谱的贡献。

DOI:
10.1021/acs.jctc.6b00279
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发表时间:
2016
影响因子:
5.5
通讯作者:
S. Mukamel
S. Mukamel
中科院分区:
化学1区
文献类型:
--
作者:
J. Rouxel;M. Kowalewski;S. Mukamel

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受激(相干)和自发(非相干)非线性X射线信号表示使用空间非局部响应张量,直接连接到时间演变的电流j和电荷σ密度,而不是电和磁多极。证明了σA(2)和j · A最小耦合项(A为矢势)的相对贡献。这两个占主导地位的非共振和共振散射,分别,并作出相当的贡献,在近共振失谐。
Stimulated (coherent) and spontaneous (incoherent) nonlinear X-ray signals are expressed using a spatially nonlocal response tensor which directly connects them to the time evolving current j and charge σ densities rather than to electric and magnetic multipoles. The relative contributions of the σA(2) and j · A minimal coupling terms, where A is the vector potential, are demonstrated. The two dominate off-resonant and resonant scattering, respectively, and make comparable contributions at near resonant detunings.
DOI: 10.1021/nl2043437
发表时间: 2012-06-01
期刊: NANO LETTERS
影响因子: 10.8
作者:
Kao, T. S.;Rogers, E. T. F.;Zheludev, N. I.
通讯作者: Zheludev, N. I.