Observation of a C-type short-range antiferromagnetic order in layer spacing expanded FeS

Observation of a C-type short-range antiferromagnetic order in layer spacing expanded FeS
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层间距扩展 FeS 中 C 型短程反铁磁序的观察

DOI:
10.1103/physrevmaterials.4.034802
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发表时间:
2020
影响因子:
3.4
通讯作者:
Birgeneau RJ
Birgeneau RJ
中科院分区:
材料科学3区
文献类型:
--
作者:
Wang M;Yi M;Frandsen BA;Yin J;Sun H;Xu Z;Cao H;Bourret-Courchesne E;Lynn JW;Birgeneau RJ

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We report neutron diffraction studies of FeS single crystals obtained from RbxFe2−yS2 single crystals via a hydrothermal method. While no iron vacancy order or block antiferromagnetic order typical of RbxFe2−yS2 is found in our samples, we observe C-type short-range antiferromagnetic order with moments pointed along the c axis hosted by a different phase of FeS with an expanded interlayer spacing. The Néel temperature for this magnetic order is determined to be 170 ± 4 K. Our finding of a variant FeS structure hosting this C-type antiferromagnetic order demonstrates that the known FeS phase synthesized in this method is in the vicinity of a magnetically ordered ground state, providing insights into understanding a variety of phenomena observed in FeS and the related FeSe1−xSx iron chalcogenide system.
通过调节 FeSe1-xSx 超导体的向列性和磁性来最大化 T-c
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