Origin of the 4.1-eV luminescence in pure CsI scintillator.

Origin of the 4.1-eV luminescence in pure CsI scintillator.
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纯 CsI 闪烁体中 4.1-eV 发光的起源。

DOI:
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发表时间:
1995
期刊:
Physical Review B (Condensed Matter)
影响因子:
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通讯作者:
Nakayama
Nakayama
中科院分区:
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文献类型:
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作者:
Nishimura;Sakata;Tsujimoto;Nakayama

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利用双光子光谱法,在宽温度范围(4.5\char21{}300 K)下,观察了与CsI中自俘获激子(STE)相关的4.3 ev和3.7 ev发光带的光谱和衰减时间。结果表明,纯CsI的4.1 eV发光,即所谓的室温闪烁,主要出现在4.3 eV的STE状态,在6 K以下以4.3 eV的STE发光为主,在6 K以上被淬灭,但在4.1 eV的室温下,由3.7 eV STE状态到4.3 eV STE状态的STE热活化再次出现。
The spectra and decay times of the 4.3- and 3.7-eV luminescence bands associated with the self-trapped excitons (STE's) in CsI have been observed in a wide temperature range (4.5\char21{}300 K) by using two-photon spectroscopy. The results reveal that the 4.1-eV luminescence in pure CsI, which is well known as the room-temperature scintillation, appears mainly from the 4.3-eV STE state: the 4.3-eV STE luminescence is dominant below 6 K and is quenched above 6 K, but appears again at 4.1 eV at room temperature by thermal activation of STE's from the 3.7-eV STE state to the 4.3-eV STE state.