Nonlinear Optical Response of Colloidal Gold Nanoparticles Studied by Hyper-Rayleigh Scattering Technique

Nonlinear Optical Response of Colloidal Gold Nanoparticles Studied by Hyper-Rayleigh Scattering Technique
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超瑞利散射技术研究胶体金纳米粒子的非线性光学响应

DOI:
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发表时间:
2000
期刊:
影响因子:
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通讯作者:
LuZuhong
LuZuhong
中科院分区:
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文献类型:
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作者:
ShenYao;TangZuming;GuiMinzhi;ChengJiqi;WangXing;LuZuhong

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利用超瑞利散射(HRS)技术研究了纳米金颗粒悬浮液的非线性光学响应。在400 nm处测得的信号强度与1064 nm处的泵浦激光能量呈三次关系,表明测量到的信号是一个三阶非线性光学过程,即三光子激发荧光(3PF)。据我们所知,这是首次对胶体金纳米颗粒悬浮液进行3PF的实验观察。
Hyper-Rayleigh scattering (HRS) technique is used to study the nonlinear optical response of nanocrystalline gold particle suspensions. The signal intensity measured at 400 nm has a cubic dependence on the pump laser energy at 1064 nm, indicating that the measured signal is due to a third-order nonlinear optical process, namely three-photon excited fluorescence (3PF). To the best of our knowledge, this is the first experimental observation of 3PF for colloidal gold nanoparticle suspensions.
DOI: 10.1126/science.2321027
发表时间: 1990-04-06
期刊: SCIENCE
影响因子: 56.9
作者:
DENK, W;STRICKLER, JH;WEBB, WW
通讯作者: WEBB, WW