Degree of molecular self-sorting in multicomponent systems
Degree of molecular self-sorting in multicomponent systems
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DOI：
10.1039/c2ob25098e
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发表时间：
2012-01-01
影响因子：
3.2
通讯作者：
Schmittel, Michael
中科院分区：
文献类型：
--
作者：
Saha, Manik Lal;Schmittel, Michael
自分选表示复杂混合物中两种或更多种相关组分的自发和高保真的自我和/或非自我识别。虽然有效管理的自我分选原则明显需要一些关键的专业知识，在分子编程，在更高的操作阶段，它是最高的利益，以指导该过程越来越高程度的自我分选。在这篇文章中，我们提出了如何引导多个组件形成自排序的多组件架构的新兴原则。为了给这类系统命名提供进一步的指导，我们建议利用一个系统的分类以及一个公式来评估它们的自分类程度（M）。
Self-sorting represents the spontaneous and high fidelity self and/or non-self-recognition of two or more related components within a complex mixture. While the effective management of self-sorting principles perceptibly requires some key expertise in molecular programming, at a higher stage of operation it is of supreme interest to guide the process to increasingly higher degrees of self-sorting. In this article, we present the emerging principles of how to guide several components toward formation of self-sorted multicomponent architectures. To provide further guidance in denominating such systems, we suggest to utilise a systematic classification as well as a formula to evaluate their degree of self-sorting (M).