Luminescence and scintillation properties of (C6H5(CH2)2NH3)2(Ba,Pb)Br4 with self-organized bi-dimensional quantum-well structures

Luminescence and scintillation properties of (C6H5(CH2)2NH3)2(Ba,Pb)Br4 with self-organized bi-dimensional quantum-well structures
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DOI:
10.7567/1347-4065/ab515d
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发表时间:
2019-12
影响因子:
1.5
通讯作者:
D. Nakauchi;N. Kawano;N. Kawaguchi;T. Yanagida
D. Nakauchi;N. Kawano;N. Kawaguchi;T. Yanagida
中科院分区:
物理与天体物理4区
文献类型:
--
作者:
D. Nakauchi;N. Kawano;N. Kawaguchi;T. Yanagida

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采用溶剂扩散法制备(C6H5(CH2)4NH3)2BaxPb1−xBr4 (x = 0、0.1、0.25和0.5)晶体,考察其闪烁性能。样品表现出光致发光和闪烁,由于激子的作用,在440 nm附近有一个尖锐的发射峰,衰变时间主要为几纳秒。137Cs伽玛射线辐照下的脉冲高度谱表明,(C6H5(CH2)2NH3)2Ba0.25Pb0.75Br4和(C6H5(CH2)2NH3)2Ba0.5Pb0.5Br4晶体的闪烁光产额约为19000 ph MeV−1。
(C6H5(CH2)4NH3)2BaxPb1−xBr4 (x = 0, 0.1, 0.25 and 0.5) crystals were prepared by the solvent diffusion method to evaluate the scintillation properties. The samples exhibit photoluminescence and scintillation with a sharp emission peaking around 440 nm due to excitons, and the decay time is dominantly several nanoseconds. The pulse height spectrum under 137Cs gamma-ray irradiation demonstrates that the scintillation light yields of (C6H5(CH2)2NH3)2Ba0.25Pb0.75Br4 and (C6H5(CH2)2NH3)2Ba0.5Pb0.5Br4 crystals are approximately 19 000 ph MeV−1.