Optimal control for suppressing wave packet spreading with strong non-resonant laser pulses
Optimal control for suppressing wave packet spreading with strong non-resonant laser pulses
复制标题
强非谐振激光脉冲抑制波包扩展的优化控制
DOI:
10.1103/physreva.104.033107
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发表时间:
2021
影响因子:
2.9
通讯作者:
K. Ohmori
中科院分区:
文献类型:
--
作者:
Y. Ohtsuki;T. Namba;H. Katsuki;K. Ohmori
We use nonlinear optimal control simulation to systematically examine how to suppress wave-packet spreading with strong nonresonant near-infrared (NIR) laser pulses through a case study of a vibrational wave packet in thestate of. As the degree of spreading of the vibrational wave packet is controllable by adjusting the pump pulse shape, the vibrational wave packet may be regarded as a prototype system to study spreading suppression by using nonresonant laser pulses. We quantitatively define spreading suppression in terms of the probability of finding the wave packet in the analytically defined, initially excited state at every vibrational period. From optimal control simulation and simulation by using model Gaussian pulse trains that mimic optimal pulses, we conclude that a simple periodic NIR pulse trainwithouthighly tuned temporal widths, amplitudes, or irradiation timings can almost perfectly stop the wave-packet spreading over a long control period, provided that the degree of spreading is not too large.