Ultrafast hot-electron dynamics observed in Pt( -)(3) using time-resolved photoelectron spectroscopy

Ultrafast hot-electron dynamics observed in Pt( -)(3) using time-resolved photoelectron spectroscopy
复制标题

使用时间分辨光电子能谱观察 Pt(-)(3) 中的超快热电子动力学

DOI:
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发表时间:
2000
影响因子:
8.6
通讯作者:
Eberhardt
Eberhardt
中科院分区:
物理与天体物理1区
文献类型:
--
作者:
Pontius;Bechthold;Neeb;Eberhardt

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Time-resolved two-photon photoelectron spectra have been measured for free Pt( -)(3) using femtosecond pulses of 1.5 eV photon energy in a pump-probe configuration. The time-dependent photoelectron distribution reveals a lifetime of optically excited states of less than 70 fs. Such an unexpected fast electron relaxation in Pt( -)(3) suggests the existence of inelastic electron-electron scattering processes in a triatomic cluster which result in a lifetime similar to those of bulk metals.